##plugins.themes.bootstrap3.article.main##

Land treatment is a method of handling wastes produced by the petroleum refining industry and others. This method allows the simultaneous treatment and final disposal of the waste. This study represent a fundamental filed investigation to follow the land treatment method for disposing of an oily sludge produce by Daura Refinery Wastewater Treatment Plant. The sludge typically consists of (84.5-86.2)% water, (4.7-5.3)% oils, and (8.4-9.25)% sediments. It is characterized by law contents of phenol, nitrogen, and heavy metals of environmental concern. Loamy sand soil land located inside Daura Refinery was selected and divided into a1-sq. meter plots. A range of sludge application rates was applied to add the sludge to (mix with) the upper 15 cm soil layer of 18 plots, whereas 6 plots left as control plots. The applications range included three applications ratios of (fresh sludge wt,  : dry soil wt.) as (1:3), (1:6), and (1:10), each of them was applied in three application intervals: weekly, monthly, and seasonally. Selection of the best application rate was made with regard to sludge degradation and land area requirements. Soil samples were tested for oil residue, heavy metals, total nitrogen, electrical conductivity, pH, and aggregate stability. The results show that, monthly (1:10) application rate caused neither considerable downward oil migration in the soil nor significant accumulation of oil, heavy metals, or salts in the soil. However, it maintained neutral soil pH and improved soil aggregate stability. Oil biodegradation in the soil was encouraged by soil weakly tillage.

Downloads

Download data is not yet available.

References

  1. Grove, G.W. ''Use landfarming for oily waste disposal''. Hydrocarbon Processing, 57: 138-140, 1978.
     Google Scholar
  2. Raymond. C.L.; ASCE, M.; and Overcash, M.R., ''Land Treatment of Wastes: Concepts and general design'', J. Environ. Engineering, 111(2): 141-160, 1985.
     Google Scholar
  3. Handdelston, R.L. ''Solid waste disposal: Landfarming'', Chemical Engineering, 86(5): 119-124, 1979.
     Google Scholar
  4. Arora, H.S.; Cantor, R.R.; and Nemeth, J.C., ''Land treatment: Available and successful method petroleum industry wastes'', Environ International., 7: 285-291, 1982.
     Google Scholar
  5. Raymond, C.L.; John, R.R.; and Rucker, J.E. '' Land Treatment is viable technology for reducing petroleum – waste toxicity and migration potential'', Oil & Gas J., 85(44): 40-43, 1987.
     Google Scholar
  6. Dotson, G.K.; Dean, R.B.; Kenner, B.A.; and cooke, W.E. ''Land spreading: A conversation and Non- polluting method of disposing of oily wastes'', 5th Intl. Water Poll. Res. Conf. and Exhib., San Francisco, CA, July 26 – Aug 1,1970. (Cited in El-Nawawy 1990).
     Google Scholar
  7. Kincannon, C.B. ''Oily waste disposal by soil cultivation process'', U.S. Govt. publication, EPA-P-72-110, Washington D.C., U.S.A.,1972. (Cited in El-Nawawy, 1990).
     Google Scholar
  8. Dibble, J.T. and Bartha, R. ''Effect of environmental parameters on the biodegradation of oily sludge'', Appl. Environ. Microbiol., 37(4): 729-739,1979.
     Google Scholar
  9. Brown, K.W.; Barwand H.; Thomas J.C.; and Evans, G.B. ''Impact of simulated land treatment with oily sludges on reyegrass emergence and yield''. Agronomy J. 74 (2): 257-261, 1982.
     Google Scholar
  10. Wilton, B.S.; Bloys, J.B.; Watts, R.D.; and Hipp, B.W., ''Drilling wastes evaluated in plant growth study'', Drilling proceedings – SPE Annual Technical Conference and Exhibition, Washington, DC. USA. 1992, Oct. 4-7, 1992.
     Google Scholar
  11. Brown, K.W. and Deuel, Jr. L.E., ''Evaluation of subsurface conditions at refinery land treatment sites'', Texas A and M Univ., College station, USA, Report no.: EPA – 600/2 – 83- 096, 1983.
     Google Scholar
  12. Bleckmann, C.A.; Gawel L.J.; Whitfill, D.L.; and Swindoll, C.M. (1989) ''Land Treatment of Oil – based drill cuttings'', SPE/IADC 1989 Drilling. Conference, New Orleans, L.A., USA, Feb. 28 – Mar 3, 1989
     Google Scholar
  13. El-Bagouri, I.H.; El-Nawawy, A.S.; Abdal, M.; Al-Daher, R.; Khalafawi M.S.; Whitton, B.A.; and Wong. Ming H. (eds) ''Mobility of oil and other sludge constitute during oily sludge treatment by landfarming'', Int. Conf. of Environmental Biotechnology in Waste Treatment and Recycling, Hong Kong, Jan. 12-14, 1994.
     Google Scholar
  14. Streebin, L.E.; Robertson, J.M.; Schornick, H.M; Bowen, P.T.; and Bagawandoss, K.M. ''Land Treatment of Petroleum Refinery Sludges'', Oklahoma Univ., Norman School of Civil Eng. And Environ. Sci., Report no. EPA/600/2-84/193, 1984.
     Google Scholar
  15. Streebin, L.E.; Robertson, J.M.; Callender, A.B.; Doty, L.; and Bagawandoss, K., ''Closure evaluation for petroleum residue land treatment'', Oklahoma U niv., Norman School of Civil Eng. And Environ. Sci., Report no. EPA/600/2-84/162, 1984.
     Google Scholar
  16. Genouw G, Naeyer F, Meenen P, Werf H, Nijs W, "Degradation of oily sludge by land farming – a case study at the Ghent Harbour". Biodegradation 5: 37-46,1994.
     Google Scholar
  17. Al-Khateeb, H.M, "Disposal of an Oily Sludge by Landfarming", M.Sc. thesis, Civil Engineering Dep., College of Engineering, University of Mustansiriya, Baghdad, Iraq,1997.
     Google Scholar
  18. Overcash, M.R.; Nutter, W.L.; Kendall, R.L.; and Wallace, J.R. ''Field and laboratory evaluation of petroleum land treatment system closure''. Earth system associates, Material, GA. Report no. EPA/600-2-85-134, 1985.
     Google Scholar
  19. Prado-Jatar M, Correa M, Rodriguez-Graw J, Carneiro M, "Oily sludge land farming biodegradation experiment conducted at a tropical site in eastern Venezuela". Waste Management and Research ,11: 97-106, 1993.
     Google Scholar
  20. Mishra S., J. Jyot, R. C. Kuhad and B. Lal, "Evaluation of Inoculum Addition to Stimulate in Situ Bioremediation of Oily Sludge Contaminated Soil", Appl. Environ. Microbial., 67, 1675-1681, 2001.
     Google Scholar
  21. Del’Arco JP, de Franca FP "Influence of oil contamination levels on hydrocarbon biodegradation in sandy sediments", Environ. Pollut. 112:515-519, 2001.
     Google Scholar
  22. Zucchi M, Anghoni L, Borin S, Brusetti L, Dietrich G, "Response of bacterial community during bioremediation of an oil polluted soil". J Appl Microbiol , 94: 248-257, 2003.
     Google Scholar
  23. Hejazi RF, Husain T, Khan FI, "Landfarming operation of oil sludge in arid region-human health risk assessment", J. Hazard. Materi. B99:287-302, 2003.
     Google Scholar
  24. Mehrashi MR, Haghighi B, Shariat M, Naseri S, Naddafi K "Biodegradation of petroleum hydrocarbon in soil". Iran. J. public Health. 32 (3):28-32, 2003.
     Google Scholar
  25. Christopher W, Kaplan, Christopher L, Kitts "Bacterial succession in a petroleum land treatment unit". Appl Environ Microbiol, 70: 1777-1786, 2004.
     Google Scholar
  26. Radetski CM, Mater L, Sperb RM, Madureira LAS, Rosin AP, Correa AXR, "Proposal of a sequential treatment methodology for the safe reuse of oil sludge-contaminated soil". J. Hazard. Mat. B ,136:967-971, 2006.
     Google Scholar
  27. Crivelaro SHR, Mariano AP, Furlan LT, Gonçalves RA, Seabra PN, Angelis DF "Evaluation of the use of vinasse as a biostimulation agent for the biodegradation of oily sludge in soil". Int. J. Brazil Biol Technol. 53(5):1217-1224, 2010.
     Google Scholar
  28. Liu W, Luo Y, Teng Y, Li Z, Ma L Q. "Bioremediation of oily sludge-contaminated soil by stimulating indigenous microbes". Environ Geochem Health. 32:23-29, 2010.
     Google Scholar
  29. Black, C.A., ''Methods of Soil Analysis, Part 1'', American Soc. Of Agronomy, Inc., Madison, Wisconsin, USA, 1965.
     Google Scholar
  30. United States Salinity Laboratory Staff, ''Diagnosis and improvement of saline and alkali soils'', Handbook 60. U.S. Govt. Printing Office, Washington, DC., USA, 1954.
     Google Scholar
  31. Black, C.A., ''Methods of Soil Analysis, Part 2'', American Soc. Of Agronomy, Inc., Madison, Wisconsin, USA. 1965
     Google Scholar
  32. Raymond, R.L.; Hudson. J.O; and Jamison, V.W.,''Oil degradation in soil'', Apple Environ Microbiol., 31 (41):522-535, 1976.
     Google Scholar
  33. Cappuccino, J.G. and Sherman, N. ''Microbiology a laboratory manual'', 2nd ed. Benjamin / Cumming Publishing Co. Inc. California, USA pp. 303, 1987.
     Google Scholar
  34. Amaral, S.P. '' Lanfarming of oily wastes: Design and Operation'', Wat. Sci. Tech., 19 (8): 75-86, 1987.
     Google Scholar
  35. Mitchell, W.W.; Loynachan, T.E.; and Mckendrick, J.D. ''Effect of tillage and fertilization on persistence of crude oil contamination in an Alaskan soil'', J. Environ. Qual., 8(4): 525-532, 1979.
     Google Scholar
  36. United States Environmental Protection Agency, ''Process design manual: Land application of municipal sludge'', EPA – 625/1-83-016, USEPA. Center for Envion. Res. Information, Cincinnati, OH, USA, 1983
     Google Scholar
  37. El-Nawawy, A.S., ''Landfarming of oily sludge: an overview''. Industerial Cooperation in The Arabian Gulf, (40): 29-46, 1990.
     Google Scholar
  38. Bolt, G.H. and Bruggenwert, M.G.M.; ed. ''soil chemistry, A. Basic Elements'', Elsevier Scientific Publishing Co., Amsterdam, the Netherlands, 1976, Pp. 173-174.
     Google Scholar
  39. Ellis, R. and Adams, R.S. ''Contaminations of soils by petroleum hydrocarbons''. Adv. Agron., 13: 197-216, 1961.
     Google Scholar
  40. Al-Khafaji, A.A.; Asker, R.S.; and Kasal, S.M. '' Effects of fuel oil on aggregate stability of a poorly structured soil form Dalmaj project'', J. Agric. Water Reso. Res., 4 (2): 83-96, 1985.
     Google Scholar